By S H Lin
This quantity provides contemporary growth and views in multi-photon approaches and spectroscopy of atoms, ions, molecules and solids. the topics within the sequence conceal the experimental and theoretical investigations within the interdisciplinary study fields of common technology together with chemistry, physics, bioscience and fabric technological know-how.
This quantity is the most recent quantity in a sequence that may be a pioneer in compiling overview articles of nonlinear interactions of photons and topic. It has made a vital contribution to the improvement and merchandising of the similar learn fields. In view of the fast progress in multi-photon strategies and multi-photon spectroscopy, care has been taken to make sure that the evaluation articles inside the sequence are readable not just by means of energetic researchers but in addition those who find themselves no longer but specialists yet intend to go into the sector.
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Extra resources for Advances in Multi-Photon Processes and Spectroscopy: (Volume 21)
This short pulse is able to do hole burning if its Franck–Condon region is smaller than the width of the wavepacket and the pulse duration is short compared to the velocity of the wavepacket. In this case, the fast and sharp laser is “perforating” the big and slow wavepacket. This behavior can be rationalized in a dressed-state picture (see also Sec. 6). In Fig. 6, the situation before (left panel), during (middle panel), and after (right panel) the laser interaction is sketched, respectively. Before the laser is turned on, a wavepacket moves on a potential, which we term V1 .
85 The electronic and vibrational wavepackets created via SFI can be probed with a separate “probe” pulse, which transfers the wavepacket between nondissociative and dissociative potentials as the pump-probe delay is varied. The measurement results are contrasted with similar data for weak-field excitation in the multiphoton regime. The ab initio calculations allow us to interpret the fragment ion yield measurements as a function of time delay in terms of vibrational wavepackets on three separate electronic states of the molecular cation.
Strong-field ionization While the interaction between a molecule and a weak electromagnetic field can be described using perturbation theory, strong-field molecular ionization is a complicated nonperturbative multi-electron process. For such processes, there are currently no complete theories which are able to predict molecular-ionization yields, even given a fairly good understanding of the molecular structure. 76, 77 Figure 7 illustrates the distortion of the atomic binding potential under the influence of a strong electric field at the peak of an oscillating laser pulse.
Advances in Multi-Photon Processes and Spectroscopy: (Volume 21) by S H Lin